A versatile setup for ultrafast broadband optical spectroscopy of coherent collective modes in strongly correlated quantum systems
نویسندگان
چکیده
A femtosecond pump-probe setup is described that is optimised for broadband transient reflectivity experiments on solid samples over a wide temperature range. By combining high temporal resolution and a broad detection window, this apparatus can investigate the interplay between coherent collective modes and high-energy electronic excitations, which is a distinctive characteristic of correlated electron systems. Using a single-shot readout array detector at frame rates of 10 kHz allows resolving coherent oscillations with amplitudes <10-4. We demonstrate its operation on the charge-transfer insulator La2CuO4, revealing coherent phonons with frequencies up to 13 THz and providing access into their Raman matrix elements.
منابع مشابه
A witness for coherent electronic vs vibronic-only oscillations in ultrafast spectroscopy.
We report a conceptually straightforward witness that distinguishes coherent electronic oscillations from their vibronic-only counterparts in nonlinear optical spectra of molecular aggregates. Coherent oscillations as a function of waiting time in broadband pump/broadband probe spectra correspond to coherent electronic oscillations in the singly excited manifold. Oscillations in individual peak...
متن کاملA ug 2 00 5 Theory of ultrafast exciton dynamics in the Quantum Hall system
We discuss a theory of the ultrafast non-linear optical response of excitons in the Quantum Hall system. Our theory focusses on the role of the low energy collective electronic excitations of the cold, strongly correlated, two–dimensional electron gas (2DEG) present in the ground state. It takes into account ground state electron correlations and Pauli exchange and interaction effects between t...
متن کاملMultidimensional coherent optical spectroscopy of semiconductor nanostructures: a review
Multidimensional Coherent optical Spectroscopy (MDCS) is an elegant and versatile tool to measure the ultrafast nonlinear optical response of materials. Of particular interest for semiconductor nanostructures, MDCS enables the separation of homogeneous and inhomogeneous linewidths, reveals the nature of coupling between resonances, and is able to identify the signatures of many-body interaction...
متن کاملElectrostatics Modes in Mono-Layered Graphene
In this paper, we investigated the corrected plasmon dispersion relation for graphene in presence of a constant magnetic field which it includes a quantum term arising from the collective electron density wave interference effects. By using quantum hydrodynamic plasma model which incorporates the important quantum statistical pressure and electron diffraction force, the longitudinal plasmons ar...
متن کاملFinding Electrostatics modes in Metal Thin Films by using of Quantum Hydrodynamic Model
In this paper, by using a quantum hydrodynamic plasma model which incorporates the important quantum statistical pressure and electron diffraction force, we present the corrected plasmon dispersion relation for graphene which includes a k quantum term arising from the collective electron density wave interference effects (which is integer and constant and k is wave vector). The longitudinal ...
متن کامل